C60 adsorption on an aperiodically modulated Cu surface

Copper deposited on the ve-fold surface of icosahedral Al-Pd-Mn forms domains of a structure whose surface has a one-dimensional aperiodic modulation. It is shown that C60 deposited on this aperiodic film has highly reduced mobility as compared to C60 deposited on periodic Cu surfaces. This fnding is explained in terms of the recently proposed structural model of this system

Radiometric calibration and processing procedure for reflective bands on LANDSAT-4 protoflight Thematic Mapper

The radiometric subsystem of NASA's LANDSAT-4 Thematic Mapper (TM) sensor is described. Special emphasis is placed on the internal calibrator (IC) pulse shapes and timing cycle. The procedures for the absolute radiometric calibration of the TM channels with a 122-centimeter integrating sphere and the transfer of radiometric calibration from the channels to the IC are reviewed. The use of the IC to calibrate TM data in the ground processing system consists of pulse integration, pulse averaging, IC state identification, linear regression analysis, and histogram equalization. An overview of the SCROUNGE-era (before August 1983) method is presented. Procedural differences between SCROUNGE and the TIPS-era (after July 1983) and the implications of these differences are discussed

Impact of the Desert dust on the summer monsoon system over Southwestern North America

The radiative forcing of dust emitted from the Southwest United States (US) deserts and its impact on monsoon circulation and precipitation over the North America monsoon (NAM) region are simulated using a coupled meteorology and aerosol/chemistry model (WRF-Chem) for 15 years (1995–2009). During the monsoon season, dust has a cooling effect (−0.90 W m<sup>−2</sup>) at the surface, a warming effect (0.40 W m<sup>−2</sup>) in the atmosphere, and a negative top-of-the-atmosphere (TOA) forcing (−0.50 W m<sup>−2</sup>) over the deserts on 24-h average. Most of the dust emitted from the deserts concentrates below 800 hPa and accumulates over the western slope of the Rocky Mountains and Mexican Plateau. The absorption of shortwave radiation by dust heats the lower atmosphere by up to 0.5 K day<sup>−1</sup> over the western slope of the Mountains. Model sensitivity simulations with and without dust for 15 summers (June-July-August) show that dust heating of the lower atmosphere over the deserts strengthens the low-level southerly moisture fluxes on both sides of the Sierra Madre Occidental. It also results in an eastward migration of NAM-driven moisture convergence over the western slope of the Mountains. These monsoonal circulation changes lead to a statistically significant increase of precipitation by up to ~40 % over the eastern slope of the Mountains (Arizona-New~Mexico-Texas regions). This study highlights the interaction between dust and the NAM system and motivates further investigation of possible dust feedback on monsoon precipitation under climate change and the mega-drought conditions projected for the future

Characterization of radiometric calibration of LANDSAT-4 TM reflective bands

Prelaunch and postlaunch internal calibrator, image, and background data is to characterize the radiometric performance of the LANDSAT-4 TM and to recommend improved procedures for radiometric calibration. All but two channels (band 2, channel 4; band 5, channel 3) behave normally. Gain changes relative to a postlaunch reference for channels within a band vary within 0.5 percent as a group. Instrument gain for channels in the cold focal plane oscillates. Noise in background and image data ranges from 0.5 to 1.7 counts. Average differences in forward and reverse image data indicate a need for separate calibration processing of forward and reverse scans. Precision is improved by increasing the pulse integration width from 31 to 41 minor frames, depending on the band

Dynamical theory for modeling dipole-dipole interactions in a microcavity: The Green dyadic approach

A dynamical theory for modeling the dipole-dipole interaction in a microcavity is formulated using the Green dyadic approach. To our knowledge, this theory is one of the most general in many aspects of modeling the phenomenon. It accommodates an arbitrary number of layers adjacent to the cavity, constant but arbitrary dielectric properties within each layer, inclusion of retardation effects, arbitrary dipole orientations, and an unlimited number of interacting dipoles. Numerical results for the emission properties of interacting molecular dipoles in a microcavity are presented to illustrate the capability of the method

Lifetime and polarization of the radiative decay of excitons, biexcitons and trions in CdSe nanocrystal quantum dots

Using the pseudopotential configuration-interaction method, we calculate the intrinsic lifetime and polarization of the radiative decay of single excitons (X), positive and negative trions (X+ and X−), and biexcitons (XX) in CdSe nanocrystal quantum dots. We investigate the effects of the inclusion of increasingly more complex many-body treatments, starting from the single-particle approach and culminating with the configuration-interaction scheme. Our configuration-interaction results for the size dependence of the single-exciton radiative lifetime at room temperature are in excellent agreement with recent experimental data. We also find the following. (i) Whereas the polarization of the bright exciton emission is always perpendicular to the hexagonal c axis, the polarization of the dark exciton switches from perpendicular to parallel to the hexagonal c axis in large dots, in agreement with experiment. (ii) The ratio of the radiative lifetimes of mono- and biexcitons (X):(XX) is ~1:1 in large dots (R=19.2 Å). This ratio increases with decreasing nanocrystal size, approaching 2 in small dots (R=10.3 Å). (iii) The calculated ratio (X+):(X−) between positive and negative trion lifetimes is close to 2 for all dot sizes considered

Wave Propagation in Gravitational Systems: Completeness of Quasinormal Modes

The dynamics of relativistic stars and black holes are often studied in terms of the quasinormal modes (QNM's) of the Klein-Gordon (KG) equation with different effective potentials $V(x)$. In this paper we present a systematic study of the relation between the structure of the QNM's of the KG equation and the form of $V(x)$. In particular, we determine the requirements on $V(x)$ in order for the QNM's to form complete sets, and discuss in what sense they form complete sets. Among other implications, this study opens up the possibility of using QNM expansions to analyse the behavior of waves in relativistic systems, even for systems whose QNM's do {\it not} form a complete set. For such systems, we show that a complete set of QNM's can often be obtained by introducing an infinitesimal change in the effective potential

Radiative impact of mineral dust on monsoon precipitation variability over West Africa

The radiative forcing of dust and its impact on precipitation over the West Africa monsoon (WAM) region is simulated using a coupled meteorology and aerosol/chemistry model (WRF-Chem). During the monsoon season, dust is a dominant contributor to aerosol optical depth (AOD) over West Africa. In the control simulation, on 24-h domain average, dust has a cooling effect (−6.11 W m⁻²) at the surface, a warming effect (6.94 W m⁻²) in the atmosphere, and a relatively small TOA forcing (0.83 W m⁻²). Dust modifies the surface energy budget and atmospheric diabatic heating. As a result, atmospheric stability is increased in the daytime and reduced in the nighttime, leading to a reduction of late afternoon precipitation by up to 0.14 mm/h (25%) and an increase of nocturnal and early morning precipitation by up to 0.04 mm/h (45%) over the WAM region. Dust-induced reduction of diurnal precipitation variation improves the simulated diurnal cycle of precipitation when compared to measurements. However, daily precipitation is only changed by a relatively small amount (−0.17 mm/day or −4%). The dust-induced change of WAM precipitation is not sensitive to interannual monsoon variability. On the other hand, sensitivity simulations with weaker to stronger absorbing dust (in order to represent the uncertainty in dust solar absorptivity) show that, at the lower atmosphere, dust longwave warming effect in the nighttime surpasses its shortwave cooling effect in the daytime; this leads to a less stable atmosphere associated with more convective precipitation in the nighttime. As a result, the dust-induced change of daily WAM precipitation varies from a significant reduction of −0.52 mm/day (−12%, weaker absorbing dust) to a small increase of 0.03 mm/day (1%, stronger absorbing dust). This variation originates from the competition between dust impact on daytime and nighttime precipitation, which depends on dust shortwave absorption. Dust reduces the diurnal variation of precipitation regardless of its absorptivity, but more reduction is associated with stronger absorbing dust